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Complexes formed in collisions between ultracold alkali-metal diatomic molecules and atoms [dataset] Open Access
We explore the properties of 3-atom complexes of alkali-metal diatomic molecules with alkali-metal atoms, which may be formed in ultracold collisions. We estimate the densities of vibrational states at the energy of atom-diatom collisions, and find values ranging from 2.2 to 350 K^{-1}. However, this density does not account for electronic near-degeneracy or electron and nuclear spins. We consider the fine and hyperfine structure expected for such complexes. The Fermi contact interaction between electron and nuclear spins can cause spin exchange between atomic and molecular spins. It can drive inelastic collisions, with resonances of three distinct types, each with a characteristic width and peak height in the inelastic rate coefficient. Some of these resonances are broad enough to overlap and produce a background loss rate that is approximately proportional to the number of outgoing inelastic channels. Spin exchange can increase the density of states from which laser-induced loss may occur.
Descriptions
- Resource type
- Dataset
- Contributors
- Creator:
Frye, Matthew D.
1
Hutson, Jeremy M. 1
1 Durham University, UK
- Funder
-
Engineering and Physical Sciences Research Council
- Research methods
- Other description
- Keyword
- Ultracold scattering
Sticky collisions
- Subject
-
Ultracold molecules
- Location
- Language
- Cited in
- doi:10.1088/1367-2630/ac3ff8
- Identifier
- ark:/32150/r2sb397829n
doi:10.15128/r2sb397829n
- Rights
- Creative Commons Attribution 4.0 International (CC BY)
- Publisher
-
Durham University
- Date Created
File Details
- Depositor
- M.D. Frye
- Date Uploaded
- 15 September 2021, 15:09:13
- Date Modified
- 20 December 2021, 12:12:21
- Audit Status
- Audits have not yet been run on this file.
- Characterization
-
File format: zip (ZIP Format)
Mime type: application/zip
File size: 1347586
Last modified: 2021:12:19 23:17:39+00:00
Filename: Data_for_repository.zip
Original checksum: 8496e463637c8b2cd40b7f9b12d14466
User Activity | Date |
---|---|
User N. Syrotiuk has updated Complexes formed in collisions between ultracold alkali-metal diatomic molecules and atoms [dataset] | almost 3 years ago |
User N. Syrotiuk has updated Complexes formed in collisions between ultracold alkali-metal diatomic molecules and atoms [dataset] | almost 3 years ago |
User M.D. Frye has updated R.txt | about 3 years ago |
User M.D. Frye has deposited R.txt | about 3 years ago |