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Ultracold Molecules for Quantum Simulation: Rotational Coherences in CaF and RbCs [dataset and software] Open Access

Polar molecules offer a new platform for quantum simulation of systems with long-range interactions, based on the electrostatic interaction between their electric dipole moments. Here, we report the development of coherent quantum state control using microwave fields in 40Ca19F and 87Rb133Cs molecules, a crucial ingredient for many quantum simulation applications. We perform Ramsey interferometry measurements with fringe spacings of ~ 1 kHz and investigate the dephasing time of a superposition of N = 0 and N = 1 rotational states when the molecules are confined. For both molecules, we show that a judicious choice of molecular hyperfine states minimises the impact of spatially varying transition-frequency shifts across the trap. For magnetically trapped 40Ca19F we use a magnetically insensitive transition and observe a coherence time of 0.61(3) ms. For optically trapped 87Rb133Cs we exploit an avoided crossing in the AC Stark shifts and observe a maximum coherence time of 0.75(6) ms.

Descriptions

Resource type
Dataset
Contributors
Creator: Blackmore, Jacob 1
Creator: Caldwell, Luke 2
Gregory, Philip 1
Bridge, Elizabeth 1
Sawant, Rahul 1
Aldegunde, Jesus 3
Hutson, Jeremy 4
Sauer, Benjamin 2
Contact person: Tarbutt, Michael 2
Contact person: Cornish, Simon 1
1 Department of Physics,Durham University, UK
2 Centre for Cold Matter, Imperial College London, UK
3 Departamento de Quimica Fisica,Universidad de salamanca,Spain
4 Department of Chemistry,Durham University, UK
Funder
Engineering and Physical Sciences Research Council
Research methods
Other description
Keyword
Ramsey Spectroscopy
Coherences
Bloch Sphere
RbCs
CaF
Laser Cooling
Quantum Simulation
Subject
Coherent states
Quantum theory--Simulations
Location
Language
Cited in
Identifier
ark:/32150/r2kp78gg386
doi:10.15128/r2kp78gg386
Rights
All rights reserved All rights reserved
Publisher
Durham University
Date Created

File Details

Depositor
J.A. Blackmore
Date Uploaded
Date Modified
14 November 2018, 11:11:34
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Characterization
File format: zip (ZIP Format)
Mime type: application/zip
File size: 6227125
Last modified: 2018:09:18 16:42:22+01:00
Filename: QSUM-Molecules for Quantum Simulation.zip
Original checksum: a69da545af51624094fcf02cc9e18031
Activity of users you follow
User Activity Date
User J.A. Blackmore has updated Ultracold Molecules for Quantum Simulation: Rotational Coherences in CaF and RbCs [dataset and software] about 6 years ago
User N. Syrotiuk has updated Ultracold Molecules for Quantum Simulation: Rotational Coherences in CaF and RbCs [dataset and software] about 6 years ago
User J.A. Blackmore has updated Ultracold Molecules for Quantum Simulation: Rotational Coherences in CaF and RbCs [dataset and software] about 6 years ago
User N. Syrotiuk has updated Ultracold Molecules for Quantum Simulation: Rotational Coherences in CaF and RbCs [dataset and software] about 6 years ago
User J.A. Blackmore has updated Ultracold Molecules for Quantum Simulation: Rotational Coherences in CaF and RbCs [dataset and software] about 6 years ago
User J.A. Blackmore has updated Ultracold Molecules for Quantum Simulation: Rotational Coherences in CaF and RbCs [dataset and software] about 6 years ago
User J.A. Blackmore has updated Ultracold Molecules for Quantum Simulation: Rotational Coherences in CaF and RbCs [dataset and software] about 6 years ago
User N. Syrotiuk has updated Ultracold Molecules for Quantum Simulation: Rotational Coherences in CaF and RbCs [dataset and software] about 6 years ago
User N. Syrotiuk has updated Ultracold Molecules for Quantum Simulation: Rotational Coherences in CaF and RbCs [dataset and software] about 6 years ago
User J.A. Blackmore has updated Data and source code for "Ultracold Molecules for Quantum Simulation: Rotational Coherences in CaF and RbCs" about 6 years ago
User J.A. Blackmore has deposited QSUM-Molecules for Quantum Simulation.zip about 6 years ago