Microwave-optical spectroscopy of Rydberg excitons in the ultrastrong driving regime [software]

Brewin, Alistair (Durham University, UK); Pritchett, Jonathon D (King's College London, UK); Wong, Horatio Q X (Durham University, UK); Gallagher, Liam A P (Durham University, UK); Potvliege, Robert M. (Durham University, UK); Clark, Stewart J (Durham University, UK); Jones, Matthew P A (Durham University, UK)

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Microwave-optical spectroscopy of Rydberg excitons in the ultrastrong driving regime [software] Open Access

We study the ultrastrong driving of Rydberg excitons in Cu2O by a microwave field. The effect of the field is studied using optical absorption spectroscopy, and through the observation of sidebands on the transmitted laser light. A model based on Floquet theory is constructed to study the system beyond the rotating wave approximation. We obtain near quantitative agreement between theory and experiment across a 16-fold range of microwave field strengths spanning from the perturbative to the deep strong driving regime. Compared to Rydberg atoms, the large non-radiative widths of Rydberg excitons leads to new behaviour such as the emergence of an absorption continuum without ionization.

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Resource type: Software
Contributors: Creator: Brewin, Alistair ¹
Contact person: Brewin, Alistair ¹
Data collector: Gallagher, Liam A P ¹
Data collector: Pritchett, Jonathon D ²
Data collector: Wong, Horatio Q X ¹
Data curator: Potvliege, Robert M. ¹
Data curator: Clark, Stewart J ¹
Data curator: Jones, Matthew P A ¹

¹ Durham University, UK
² King's College London, UK
Funder: Engineering and Physical Sciences Research Council
Research methods
Other description
Keyword: Rydberg excitons
Strong driving
Ultrastrong driving
Ultrastrong coupling
Floquet theory
Microwave-optical conversion
Cuprous oxide
Subject: Physics--Software
Location
Language
Cited in: arxiv:2406.18674
Identifier: ark:/32150/r25q47rn767
doi:10.15128/r25q47rn767
Rights: Creative Commons Attribution 4.0 International (CC BY)
Publisher: Durham University
Date Created

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