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Robust Storage Qubits in Ultracold Polar Molecules [dataset] Open Access

Quantum states with long-lived coherence are essential for quantum computation, simulation and metrology. The nuclear spin states of ultracold molecules prepared in the singlet rovibrational ground state are an excellent candidate for encoding and storing quantum information. However, it is important to understand all sources of decoherence for these qubits, and then eliminate them, in order to reach the longest possible coherence times. Here, we fully characterise the dominant mechanisms for decoherence of a storage qubit in an optically trapped ultracold gas of RbCs molecules using high-resolution Ramsey spectroscopy. Guided by a detailed understanding of the hyperfine structure of the molecule, we tune the magnetic field to where a pair of hyperfine states have the same magnetic moment. These states form a qubit, which is insensitive to variations in magnetic field. Our experiments reveal a subtle differential tensor light shift between the states, caused by weak mixing of rotational states. We demonstrate how this light shift can be eliminated by setting the angle between the linearly polarised trap light and the applied magnetic field to a magic angle of 55 degrees. This leads to a coherence time exceeding 5.6s at the 95% confidence level.

Descriptions

Resource type
Dataset
Contributors
Creator: Gregory, Philip David 1
Contact person: Gregory, Philip David 1
Data collector: Gregory, Philip David 1
Contact person: Cornish, Simon 1
1 Durham University, UK
Funder
Engineering and Physical Sciences Research Council
Research methods
Production and optical trapping of ultracold RbCs molecules
Ramsey spectroscopy
Other description
Keyword
Qubits
RbCs
Ultracold polar molecules
Subject
Location
Language
Cited in
doi:10.1038/s41567-021-01328-7
Identifier
ark:/32150/r25m60qr93w
doi:10.15128/r25m60qr93w
Rights
Creative Commons Attribution 4.0 International (CC BY)

Publisher
Durham University
Date Created

File Details

Depositor
P.D. Gregory
Date Uploaded
Date Modified
15 September 2021, 09:09:44
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File format: zip (ZIP Format)
Mime type: application/zip
File size: 228063
Last modified: 2021:07:02 10:17:22+01:00
Filename: DOI.zip
Original checksum: 662fc26235e2e0dccec811abcbf421e5
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