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Muon spectroscopy investigation of anomalous dynamic magnetism in NiI2 [dataset] Open Access
We present the results of muon-spin relaxation ($\mu^{+}$SR) measurements of the van der Waals magnet NiI$_2$, which probe magnetic phase transitions at $T_{\mathrm{N1}}=73$~K and $T_{\mathrm{N2}}=62$~K. Supporting density functional theory (DFT) calculations allow the determination of a single muon stopping site whose magnetic environment is consistent with the proposed ground-state magnetic structure. $\mu^{+}$SR measurements of the dynamics reveal behavior consistent with spin-wave excitations below $T_{\mathrm{N2}}$. In the region $T_{\mathrm{N2}}<T<T_{\mathrm{N1}}$ the character of the dynamics changes qualitatively, resulting in an unusual region of temperature-independent fluctuations.
Descriptions
- Resource type
- Dataset
- Contributors
- Creator:
Breeze, Theodore L.
1
Creator: Huddart, Benjamin M. 2
Creator: Hernández-Melián, Alberto 3
Creator: Bentley, Nathan P. 1
Creator: Mayoh, Daniel A. 4
Creator: Wood, George D. A. 5
Creator: Balakrishnan, Geetha 4
Creator: Wilkinson, John 5
Creator: Pratt, Francis L. 5
Creator: Hicken, Thomas J. 6
Creator: Clark, Stewart J. 1
Creator: Lancaster, Tom 1
1 Durham University
2 University of Oxford
3 Southampton University
4 Warwick University
5 ISIS
6 Swiss muon source
- Funder
-
Engineering and Physical Sciences Research Council
- Research methods
- Other description
- Keyword
- muon spin spectroscopy
Van der Waals magnets
DFT
Crystal field splitting
- Subject
-
Magnetism
Dynamics
- Location
- Language
- Cited in
- doi:10.1103/PhysRevB.111.104420
- Identifier
- ark:/32150/r1pn89d6605
doi:10.15128/r1pn89d6605
- Rights
- Creative Commons Attribution 4.0 International (CC BY)
- Publisher
-
Durham University
- Date Created
File Details
- Depositor
- T. Lancaster
- Date Uploaded
- 4 March 2025, 10:03:43
- Date Modified
- 6 February 2026, 11:02:44
- Audit Status
- Audits have not yet been run on this file.
- Characterization
-
File format: zip (ZIP Format)
Mime type: application/zip
File size: 268340
Last modified: 2026:01:30 10:34:29+00:00
Filename: NiI2_data_availability.zip
Original checksum: e90e77990f27f8b81725ce70d7cc2b71
